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Experimental possibilities of research fast reactor BOR-60

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Experimental possibilities of research fast reactor BOR-60 Efimov V.N., Zhemkov I.Yu., Korolkov A.S. FEDERAL STATE UNITARY ENTERPRISE STATE SCIENTIFIC CENTER – PowerPoint PPT presentation

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Title: Experimental possibilities of research fast reactor BOR-60


1
Experimental possibilities of research fast
reactor BOR-60
  • Efimov V.N., Zhemkov I.Yu., Korolkov A.S.
  • FEDERAL STATE UNITARY ENTERPRISE STATE SCIENTIFIC
    CENTER
  • OF RUSSIAN FEDERATION RESEARCH INSTITUTE OF
    ATOMIC REACTORS

2
  • Research fast reactor BOR-60 is one of the
    leading experimental facilities of the country
    and of the world intended for testing of a
    variety of fuel, absorbing and structural
    materials that are offered for creation of
    advanced fast, pressurized water, gas-cooled and
    fusion reactors and serving for substantiation of
    the VVER and BN-type reactor service life
    extension. The reactor has been in effective and
    reliable operation for more than 35 years already
    and at present it is practically the only
    research fast reactor that, apart from well
    equipped material science laboratories and
    pilot-scale production engaged in fuel
    fabrication and reprocessing, has unique
    experimental possibilities for complex
    investigation activities in different research
    lines.

3
Table 1 Some physical characteristics of the
reactor
Characteristic Value
Reactor heat power, MW 60
Inlet temperature of coolant, ?? 310-330
Outlet temperature of coolant, ?? 530
Fuel UO2 or UO2-PuO2
235U enrichment, 45-90
Maximum Pu concentration, 40
Maximum volumetric power in the core, kW/l 1100
Maximum neutron flux density, cm-2s-1 3.71015
Average neutron energy, MeV 0.4
Neutron fluence per 1 year, cm-2 31022
Damage dose accumulation rate, dpa/y Up to 25
Fuel burnup rate, /y Up to 6
Power non-uniformity factors Axial Radial 1.14 1.15
4
Fig. 1. Simplified schematic diagram of the
BOR-60 reactor facility
1 - reactor 2 - intermediate heat exchanger 3
- circulating pump of the first circuit 4 -
steam generator 5 - sodium-air heat
exchanger 6 - circulating pump of the second
circuit 7 - blow fan 8 - turbine 9 - turbine
condenser 10 - deaerator 11 - condensate
pumps 12 - feed pumps 13 - low pressure
heater 14-high pressure heater
5
Fig. 2. The BOR-60 reactor section
1 inlet branch pipe, 2 high pressure
chamber, 3 basket, 4 thermal and neutron
reactor vessel shielding, 5 protective
casing, 6 support flange, 7 refueling
channel, 8 driving mechanism of the control and
safety rods, 9 support flange, 10 large
rotating plug, 11 small rotating plug, 12
core and reflector assemblies
6
Fig. 3. Pressure plenum
  • 1 pressure plenum chamber
  • 2 throttle plug
  • 3 adjustable plug
  • 4 inlet chamber
  • 5 inlet chamber bottom
  • 6 - throttle
  • 7 - throttle
  • 8 - throttle
  • 9 - gasket
  • 10 shell with displacers
  • 11 - displacer

7
Fig. 4. Cartogram of the BOR-60 reactor
Reactor loading possibility
Cells quantity for S/A for absorbing rods instrumented cells 265 156 7 3
State S/A quantity 85-124
Maximum quantity of the experimental non-fuel S/A in the core 12
Maximum quantity of the experimental fuel S/A in the core 156
8
Fig. 5. Radial distribution of average neutron
energy (En), integral energy (Fn) and neutron
flux density with ?gt0.1 Mev (Fn(0.1))
9
Fig. 6. Neutron spectrum of the BOR-60 reactor
core - layer (cell number)
10
Fig. 7. Neutron spectrum of the BOR-60 reactor
reflector layer (cell number)
11
  • - For instrumented irradiation a special
    thermometric channel is used allowing allocating
    experimental devices directly in the core (D23).
    The lower part of the experimental device looks
    like a standard S/A (a fixture and a hexagonal
    tube of 44 mm of across flats dimension).
  • - In two cells (?43 and D35) it is possible to
    display limited data (thermocouples, neutron
    sensors, etc.).
  • - Peripheral cell G01 of the reflector is
    shielded by three assemblies with zirconium
    hydride that allowed mitigating the cell neutron
    spectrum and using it for radioisotope production
    and other purposes.
  • - The reactor is equipped with a horizontal (HEC)
    and 9 vertical (VEC) channels outside of the
    reactor vessel. The channels are used mainly for
    irradiation of electro technical materials and
    silicon radiation doping. By the results of the
    HEC neutron physical characteristics study it was
    concluded that the channel can be used for
    medical investigations.

12
Table 2Testing conditions of materials and
products in cell D-23
Parameter Value
Neutron flux density, sm-2s-1 21015
Specific radiation energy release in structural materials (with atomic number Z  26?30), W/g 4
Absorbed gamma-radiation dose rate, Gy/s 4.5103
Coefficient of non-uniform radiation density distribution along the core height (450 mm) for neutrons for gamma-radiation 1.13 1.25
Sodium flow rate, m3/h when fed from high pressure chamber when fed from low pressure chamber up to 8 up to 2
13
Table 3 Neutron-physical characteristics of the
BOR-60 instrumented cells (Wreactor55 MW)
Cell, row Cell, row ?31, 1 ?43, 3 D23, 5 D35, 8
Radius of the cell center location against the core center, mm Radius of the cell center location against the core center, mm 45 135 196 360
Neutron flux density, 1015 sm-2s-1 Egt0.0 MeV (F0) Egt0.1 MeV (F0.1) Neutron flux density, 1015 sm-2s-1 Egt0.0 MeV (F0) Egt0.1 MeV (F0.1) 3.4 2.8 3.1 2.5 2.5 2.0 1.2 0.6
Damage accumulation rate in steel (DPA), 10-6 d.p.a./s Damage accumulation rate in steel (DPA), 10-6 d.p.a./s 1.4 1.3 1.0 0.2
Kz(AP), relative unit F0 1.15 1.16 1.15 1.12
Kz(AP), relative unit F0.1 1.17 1.17 1.17 1.15
Kz(AP), relative unit DPA 1.18 1.18 1.18 1.16
Kr(CCP), relative unit F0 1.00 1.05 1.09 1.13
Kr(CCP), relative unit DPA 1.01 1.06 1.11 1.31
Neutron flux density fraction with energy exceeding 0.1 MeV, relative unit Neutron flux density fraction with energy exceeding 0.1 MeV, relative unit 0.83 0.82 0.80 0.50
Average neutron energy, keV Average neutron energy, keV 350 320 250 40
Neutron fluence, 1022 sm-2 Egt0.0 MeV 5.5 5.0 4.1 1.9
Neutron fluence, 1022 sm-2 Egt0.1 MeV 4.6 4.1 3.3 1.0
Steel damage dose, d.p.a. Steel damage dose, d.p.a. 24 21 17 4
1 year of irradiation - WT 250 000 MWh, Kz and
Kr axial and radial non-uniformity coefficient.
14
Fig. 8. Neutron spectrum of cell G01 of the
BOR-60 reflector
15
Fig. 9. BOR-60 HEC and VEC location scheme
1 - HEC, 2 - sand, 3 - oxide, 4 disperser
drive, 5 cast iron, 6 - graphite, 7 -
concrete, 8 - VEC
16
Fig. 10. Neutron spectrum of the BOR-60 VEC
(calculations were made on the basis of MMK and
OKS-ROZ-6 programs)
17
Fig.11. Neutron spectrum at the HEC inlet and
outlet
Table 4 Neutron flux and gamma-quantum density at
the BOR-60 HEC outlet (sm-2s-1)
HEC  Calculated value Calculated value Experiment value
HEC  Fn Fg Fn
Without Pb-screen, ?ngt0 MeV (0.84?1.2)?1010 9.6?108 (2.9?3.4)?108
Without Pb-screen, ?ngt1.2 MeV (6.2?8.6)?107 - (5.7?6.5)?107
With Pb-screen 3.6?109 2.9?106 -
18
Fig. 12. Typical diagram of the BOR-60 reactor
operation
19
  • Long term investigation of neutron physical,
    heat-hydraulic and dynamic reactor
    characteristics allowed detailed study of reactor
    behavior in different operation modes, creating a
    complex of computation programs for reactor
    operation and experiments performance. As a
    result, calculations authenticity increased to
    support experimental programs, reactor operation
    and its safety substantiation. On the basis of
    great experience of reactor characteristics
    investigations and a verified complex of
    computation programs different methods were
    developed that enable high accuracy control of
    operation modes and parameters of materials
    irradiation in the non-instrumented reactor
    cells.

20
Table 5 Irradiation parameters errors,
Parameter Measurement Calculation
Intel (outlet) reactor temperature 1,2 -
Reactor power - 2,5
Reactor flow rate 3 -
Neutron flux (fluence) 7 10
Experimental devices (ED) flow rate 2 -
ED power 7 10
Intel ED temperature 1 1,5
Outlet ED temperature 1 1-3
21
  • For irradiation of a variety of materials and
    products at different operation modes and
    parameters a complex of specialized test devices
    is used. The test devices consist of capsule
    devices, dismountable material science
    assemblies, autonomous instrumented channels,
    special instrumented S/As etc.
  • Simple design of the devices and possibility to
    install them practically into any core or
    reflector cell can be considered an undoubted
    advantage of the devices.
  • The main task the developer of the test devices
    faces is creation of the required temperature
    modes at the specimens. For this purpose thermal
    insulating clearances, intensive cooling or
    additional heating due to radiation energy
    release or fuel fission are used. Temperature
    stabilization is achieved as a result of
    thermistor change in the scheme of heat transfer
    due to the coolant temperature change or as a
    result of the heat removal intensification by
    using liquid metal under boiling condition. These
    devices help to provide the specified axial and
    azimuthal temperature non-uniformity.

22
Fig. 13. Flow experimental assemblies
Fig. 14. Device with evaporativewith gas heat
insulation
thermosiphon
1 specimens 2 shell 3 heater 4 body
1,2 outer and inner bodies 3 clearance 4
shells 5 - specimens
23
The lower boundary of the irradiation temperature
range that is ensured in the BOR-60 reactor makes
up 300-310??. It significantly expands the scope
of reactor work, including experiments on
investigation of physical and mechanical
properties of zirconium alloys and materials of
the VVER-type reactor internals. At relatively
high coolant flow rate the dismountable assembly
allows irradiating structural materials specimens
at the temperature close to the reactor inlet
temperature. This assembly is one of the simplest
and widely used experimental devices helping to
perform intermediate reloading procedures and
investigation of specimens with their subsequent
irradiation. The dismountable assembly is also
used for irradiation of fuel elements.
1 - thermometric probe 6 - gas clearance 2 -
detachable head 7 - inner pipe 3 - spacer
tubes 8 - capsule assembly 4 - probe
thermocouples 9 - core center 5 - wrapper 10
- fixture
  • Fig. 15. Dismountable assembly with a hot probe
    for irradiation of
  • structural materials

24
1, 2 leak-tight capsules with different type
specimens in lithium-4 medium 3 inner capsule
cladding from Inconel-type heat-resistant
steel 4 outer capsule cladding from stainless
steel 5 ampoule sodium 6 ampoule
clearance 7 leak-tight wrappers from
Inconel-type heat-resistant steel with
thermocouples
  • Fig.16. Cross-section of the experimental device
    with capsules for irradiation of vanadium in
    lithium medium

25
  • 1 - fixture
  • 2 - throttling orifice
  • 3 - filter
  • 4 - block of tungsten rods
  • 5 - gas clearance
  • 6 - block of steel rods
  • 7 - head
  • Fig. 17. Scheme of sodium boiling generator

26
1 fuel assembly 2 - nozzle body 3 tube with
sensors 4 flow regulator 5 sodium vapor
filter 6 electric engine
  • Fig. 18. Scheme of the instrumented nozzle

27
1 sodium vapor catcher 2- level gauges inside
of the channel 3 maximum sodium level in the
channel 4- KGO pipe 5 sodium flow regulator 6
sodium yield from electromagnetic pump 7 MGD
pump 8 fuel assembly body 9 sodium upflow in
the channel 10 sodium down flow in the channel
11- upflow of reactor sodium 12 heat
insulating gas clearance of FA in the channel 13
channel body 14 - neutron sensors 15 inner
wrapper of the channel 16 fuel elements 17
membrane 18 tube for sodium channel filling 19
throttling orifice 20 channel tail 21 inlet
of reactor sodium into the channel from the
BOR-60 high pressure chamber 22 protective
membrane 1-8 thermocouples
Cross-section of the loop channel core center
  • Fig. 19. Scheme of the capsule loop with the
    MGD-pump

28
ILCC cross-section in the core central plane
Fig. 20. Scheme of the lead loop
29
Main directions of investigation
  • - Study of safety issues. A series of experiments
    on substantiation of fast sodium reactor safety
    was performed. Among them are feeding of gas
    into the core, sodium boiling, blocking of
    coolant flow in the experimental FA resulting in
    fuel elements damage, intercircuit leaks in steam
    generators etc. Detailed study of different
    normal and off-normal processes at the BOR-60
    reactor allowed testing and adjusting of methods
    and means of abnormities diagnostics.
  • - Testing of fuel, absorbing and structural
    materials. Irradiation programs are paid special
    attention to, among them
  • Mass testing of fuel elements and fuel assemblies
    up to the burn up of 30 h.a. under steady-state
    and transition conditions
  • Testing of different neutron absorbing materials
  • Radiation testing of structural reactor
    materials
  • Testing of electric insulating, magnetic and
    refractory materials for fussion reactors

30
  • Investigations in radiation material science
  • Determination of deformation, long-term strength
    and fracture toughness dependence at temperature
    of 320-1000?? up to the dose of 200 dpa
  • Study of the technology of long-lived
    radionuclides transmutation and burning out from
    spent fuel of different reactors
  • Radiation silicon alloying for radio electronics.
  • In 1981 fuel elements with vibropacked fuel
    columns on the basis of power-generated plutonium
    were applied for the reactor core for the first
    time. Positive results of mass testing of fuel
    elements with vibropacked uranium-plutonium oxide
    fuel in the BOR-60 reactor up to the burn up of
    more than 30, as well as of 6 experimental fuel
    assemblies up to the burn up of 9,6 in the
    BN-600 reactor can serve a real basis for
    large-scale experiments in fast power reactors to
    increase their efficiency and to enhance their
    safety.

31
  • Testing of fuel elements containing weapon grade
    plutonium-based fuel was started in 1998. 
  • In the frame of the program on development of
    closed fuel cycle elements much is being done on
    burning out and transmutation of plutonium and
    minor actinides (MA). Design-experiment
    investigations and analysis of the isotope
    content of microcapsules (40 pieces) with
    different MA sets irradiated in the BOR-60
    reactor were performed. The obtained
    design-experiment results can be used for
    adjustment of physical constants.

32
  • Results on investigation of different fuel
    compositions serve the basis for development of a
    fuel cycle of advanced fast reactors with
    enhanced safety. Among these is the BREST-OD-300
    reactor with lead coolant and nitride fuel.
  • The first stage of testing of BREST-OD-300 pilot
    fuel elements took place at the BOR-60 reactor.
  • Short-cut testing of different structural
    materials is carried out
  • Steels used for fabrication of vessel internals
    (VI) for VVER reactors
  • Zirconium alloys for VVER cores
  • Vanadium-based alloys in lithium medium for
    fusion reactors
  • Graphite for RBMK reactors.

33
Table 6Reactor materials tested in the BOR-60
reactor
Material Material Type
Fuel Ceramics UO2, UO2-PuO2, UC, UN, UPuN, UPuCN
Fuel Metal U, UPu, UpuZrNb
Fuel Ceramal U-PuO2, UO2-U, UN-U
Absorbing Samples Ta, Hf, Dy, Sm, Gd, AlB6, AlB12, EuO3
Absorbing CPS rods CrB2, B4C, Eu2O3, Eu2O3H2Zr
Structural Stainless steels OX18H9, X18H10T, ??-450, ??-823 03?16?9?2, ??-912, ??-847, ??-172, ??-68, ??-24
Structural High-nickel alloys ??-16, ?20?45?4?, ???
Structural Refractory materials V, W, Mo, Nb
Structural Zirconium alloys ?-110, ?-635, ?-125
Structural Graphites ???-2-125, ??6-6, ??-280, ???, IG-11, ???
34
Material Material Type
Electrotechnical Insulation Al2?3, SiO2, Si, mica
Electrotechnical Cables ????, ????(?)
Electrotechnical Magnets ????
Others Special ceramics ??-7, ??-46, ???, LiNbO3
Others Biological shielding materials Concretes
35
Isotope accumulation for medical purposes
  • Taking into account physical peculiarities of a
    fast reactor, commercial radionuclide
    accumulation parameters were investigated. The
    radionuclides were produced by the threshold
    neutron reactions 32P, 33P, 35S, 89Sr (reaction
    (n, ?)) and 117mSn (reaction (n,n')). Besides,
    indices of the 153Gd radionuclide accumulation
    process were also determined. The radionuclide
    was produced by reaction of radiation neutron
    capture (n,?) in the BOR-60 irradiation cells
    with specially heated neutron spectrum. At
    present serial production of strontium-89 from
    yttrium targets (for production of strontium-89
    without carrier preparation) and gadolinium-153
    from europium targets is realized for production
    of sources and preparations.

36
Plans for future reactor facility operation
  • The BOR-60 reactor has been in operation for 35
    years already, the design service life makes up
    20 years and calculated life is equal to 40
    years. Decision on possible reactor service life
    extension was made up taking into account the
    equipment and materials state, strength of the
    equipment and sodium circuit pipelines these
    are the components that contribute much to the
    reactor safety and that were fabricated in
    accordance with the current calculation norms.
    Long-term plans concerning the above mentioned
    problems are made for several decades.
  • There are plans on reactor reconstruction aiming
    at the reactor service life extension for not
    less than 30 years in comparison with the
    calculated resource. During reconstruction it is
    important to expand the reactor experimental
    possibilities and to enhance its safety. A draft
    design of a new reactor has been prepared already
    and at present design work on installation of a
    new reactor within the operating reactor facility
    is being in process.

37
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